Ultrafast Optical Excitation of a Combined Coherent-Squeezed Phonon field in SrTiO3.

نویسندگان

  • G Garrett
  • J Whitaker
  • A Sood
  • R Merlin
چکیده

We have simultaneously excited a coherent and a squeezed phonon field in SrTiO3 using femtosecond laser pulses and stimulated Raman scattering. The frequency of the coherent state (a 1.3 THz) is that of the A1g-component of the soft mode responsible for the cubic-tetragonal phase transformation at approximately 110 K. The squeezed field involves a continuum of transverse acoustic phonons dominated by a narrow peak in the density of states at a 6.9 THz.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Directly observing squeezed phonon states with femtosecond x-ray diffraction.

Squeezed states are quantum states of a harmonic oscillator in which the variance of two conjugate variables each oscillate out of phase. Ultrafast optical excitation of crystals can create squeezed phonon states, where the variance of the atomic displacements oscillates due to a sudden change in the interatomic bonding strength. With femtosecond x-ray diffraction we measure squeezing oscillati...

متن کامل

Coherent Excitation of Optical Phonons in GaAs by Broadband Terahertz Pulses

Coherent excitation and control of lattice motion by electromagnetic radiation in optical frequency range has been reported through variety of indirect interaction mechanisms with phonon modes. However, coherent phonon excitation by direct interaction of electromagnetic radiation and nuclei has not been demonstrated experimentally in terahertz (THz) frequency range mainly due to the lack of THz...

متن کامل

Coherent phonon excitation in bismuth

Ultrafast time-resolved reflectivity of a bismuth thin film evaporated on a silicon substrate is measured to investigate coherent phonons in bismuth. The reflectivity result is analyzed by a linear chirp approximation to obtain the time dependent frequencies of coherent phonons. Not only the optical modes are detected, which are generated by a combination of impulsive stimulated Raman scatterin...

متن کامل

Quantifying electron-phonon coupling in CdTe12xSex nanocrystals via coherent phonon manipulation

We employ ultrafast transient absorption spectroscopy with temporal pulse shaping to manipulate coherent phonon excitation and quantify the strength of electron-phonon coupling in CdTe1 xSex nanocrystals (NCs). Raman active CdSe and CdTe longitudinal optical phonon (LO) modes are excited and probed in the time domain. By temporally controlling pump pulse pairs to coherently excite and cancel co...

متن کامل

Origin of coherent phonons in Bi2Te3 excited by ultrafast laser pulses

Femtosecond laser pulses are used to excite coherent optical phonons in single crystal Bi2Te3 thin films. Oscillations from lowand high-frequency A1g phonon modes are observed. A perturbation model based on molecular dynamics reveals various possibilities of phonon generation due to complex interactions among different phonon modes. In order to elucidate the process of phonon generation, measur...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Optics express

دوره 1 12  شماره 

صفحات  -

تاریخ انتشار 1997